STATISTICAL ANALYSIS OF RADON CONCENTRATION IN BOREHOLE WATERS; CORRELATION TO GEOLOGICAL FORMATIONS KATSINA STATE, NORTH WESTERN NIGERIA

  • M. Abdulkadir
  • N. N. Garba
  • N. Rabiu
  • C. A. C. Abdallah
  • M. A. Saleh
  • I. M. Abdullahi
  • Aminu Saidu
  • A. Abdulkadir
Keywords: Radon Concentration, Dose estimation, Geological Formations, Katsina State

Abstract

Radon in borehole water serves as a source of natural radioactivity exposure through indoor air. Determination of naturally occurring radionuclides concentration in ground and surface waters is useful as a contribution to environmental health studies. In this research, statistical analysis of radon concentration in (borehole) water was conducted in Katsina state. The aim of this study is to analyse statistically the concentration of radon in borehole water in Katsina state and to establish a possible relationship between radon activity concentration in borehole water and underlying rock types. A total of 110 water samples were collected and analysed using Tri-carb 1000 Liquid Scintillation Counter (LSC) at the Centre for Energy Research and Training, Ahmadu Bello University. The overall average concentration of 222Rn was found to be 69 ± 3 Bql-1 with geological formations, G8 and G7 having the highest and lowest concentrations with values of 75 ± 10 Bql-1 and 57 ± 4 Bql-1 respectively, which are higher than the world average values of 10 Bql-1 set by WHO and 11.1 Bql-1 set by USEPA. The results showed that radon concentrations are clearly correlated to rock types with acidic intrusive rocks associated with values which sedimentary rocks are associated with lower concentrations.

References

Abba, L., Nasiru, R., Garba, N. N. and Ahmed, Y. A. (2020) Assessment of Annual Effective Dose Due to Inhalation and Ingestion of Radon in Water Samples from the Cement Industrial Area of Sokoto, North-Western Nigeria FUDMA Journal of Sciences (FJS)Vol. 4 No. 2, pp 615 – 619DOI: https://d oi.org/10.33003/fjs-2020-0402-172 DOI: https://doi.org/10.33003/fjs-2020-0402-172

Akinnagbe, D.M., Orosun, M.M., Orosun, R.O. Osanyinlusi, O., Yusuk, K.A., Akinyose, F.C., Olaniyan, T.A., Ige, S.O. (2018). Assessment of Radon concentration of ground water in Ijero Ekiti, Manila J. Sci. 11:32–41.

Adetoro W.A, Bello A., Yakubu3 A., Sununu S.T., Usman A., Sulieman M. (2021) Investigation of Radon Concentration in Drinking Water in Some Selected Areas of Sokoto, Nigeria International Journal of Scientific Research in Physics and Applied Sciences Vol.9, Issue.6, pp.86-91

Aruwa, A., Kassimu, A.A., Gyuk, P., Ahmadu, B and Aniegbu, J. (2017). Studies on radon concentration in underground water of Idah, Nigeria. International journal of research Granthaalayah, 5(9). DOI: https://doi.org/10.29121/granthaalayah.v5.i9.2017.2242

Banks, D., Frengstad, B., Midtgård, A. K., Jan, R. K. and Strand, T. (1998). The Chemistry of Norwegian Groundwaters: I. The Distribution of Radon, Major and Minor Elements in 1604 Crystalline Bedrock Groundwaters. Sci. Total Environ. 222, 71– 91. DOI: https://doi.org/10.1016/S0048-9697(98)00291-5

Bello, S., Kamba, A.M., and Okunade,, I.O. (2016). Radon measurement in commercial borehole waterfrom some selected areas of Kaduna metropolis using liquid scintillation counter, Int. J. Math. Phys. Sci. Res. 3 (2)71–81.

Bello, S., Nasiru, R., Garba, N. N., and Adeyemo, D. J. (2020). Annual effective doses associated with radon, gross alpha and gross beta radioactivity in drinking waterv from Shanono and Bagwai, Kano State, Nigeria. Microchemical Journal,154:104551. DOI: https://doi.org/10.1016/j.microc.2019.104551

Bonotto, D.M., Andrews, J.N., (1999). The transfer of radon and parent nuclides 238U and 234U from soils of Mebdip hills area, England, to the water phase. J. Geochem. Explor. 66, 255–268. DOI: https://doi.org/10.1016/S0375-6742(99)00016-3

Bunger, T., and Ruhle, H. (1994). Rapid procedure for determining radon-222 in drinking water H-Rn-222-TWASS- 01. Federal coordinating office for drinking water, groundwater, wastewater, sludge, waste and wastewater of nuclear power plants. ISSN 1865-8725.

Garba, N.N (2011). Determination of radon concentration in water sources of Zaria and environs using liquid scintillation counter. Unpublished M.Sc. thesis, Ahmadu Bello University, Zaria.

Garba, N.N., Rabi'u, N. Dewu B.B.M., (2012). Preliminary studies on 222Rn concentration in ground water from Zaria, Nigeria, J. Phys. Sci. 23 (1) (2012) 57–64.

Hess, C.T., Michael, V.A., Edward, B.L., Guillemette, (1990). Radon transferred from drinking water into house air. In: Cothern, C.R., Rebers, P.A. (Eds.), Radon, Radium and Uranium in Drinking Water. Lewis Publishers, Chelsea, pp. 51–67.

Hess, C.T., Michel, J., Horton, T.R., Richard, H.M., Coniglio, W.A., (1985). The occurrence of radioactivity in public water supplies in the United States. Health Phys. 48, 553. DOI: https://doi.org/10.1097/00004032-198505000-00002

ICRP (2007). 2006 Recommendations of the International Commission on Radiological Protection, ICRP Publication 103, Pergomon Press, Oxford, pp 69-72

Isam S. M. M, Pettersson, H. B. L., and E. Lund, E., (2002). Uranium and thorium series radionuclides in drinking water from drilled bedrock wells: correlation to geology and bedrock radioactivity and dose estimation Radiation Protection Dosimetry Vol. 102, No. 3, pp. 249–258 DOI: https://doi.org/10.1093/oxfordjournals.rpd.a006093

Isam, S. M. M. (2000). Radon in Natural Waters Analytical Methods; Correlation to Environmental Parameters; Radiation Dose Estimation and GIS Application. Unpublished PhD Thesis

ISO 13164-3 (2013). Water Quality - Radon-222- Part 1-3, International Organization for Standardization, Geneva,

Joseph, E. Atsue, T. and Adam, S. (2018) Assessment of Radon in Some Selected Water

Sources at Dutsinma town, Dutsinma Local Government Area Katsina State. Journal of Scientific and Engineering Research 5(5) Pg49-59

Mostafa, M.; Olaoye, M.A.; Ademola, A.K.; Jegede, O.A.; Saka, A.A.; Khalaf, H. (2022)

Measurement of Radon Concentration in Water within Ojo Axis of Lagos State, Nigeria. Analytica 3, 325–334. https://doi.org/10.3390/ DOI: https://doi.org/10.3390/analytica3030023

Misdaq M.A. and Elharti A (1997). Study of the influence of the lithological and hydrogeological parameters of aquifers on the radon emanation from underground waters using solid state nuclear track detectors. Journal of Radioanalytical and Nuclear Chemistry; 218 (2), 209-214. DOI: https://doi.org/10.1007/BF02039336

Pourhabib Z, Binesh A, Mohammadi S (2012). Evaluation of heavy radioactive radon and radium in rivers and drinking water in the Ramsar area by Parrasi. Iranian Journal of Physics Research, 11(4): 197-202.

Stein, L., (1983). The chemistry of radon. Radiochim. Acta 32, 163–171. DOI: https://doi.org/10.1524/ract.1983.32.13.163

Sun, H., Senkow, T.M., (1998). Mobilisation of thorium, radium and radon radionuclides in groundwater by successive alpha recoils. J. Hydrol. 205, 126–136. DOI: https://doi.org/10.1016/S0022-1694(97)00154-6

Suomela, J. (1993). Method for determination of Rn-222 in water by liquid scintillation counting according to ISO/TC147/SC3/WG6/working document N14. ISSN.0282- 4434.

Tabar, E,. Yakut, H., (2014). Radon measurements in water samples from the thermal springs of Yalova basin, Turkey, J. Radioanal. Nucl Chem. 299(1)311–319. DOI: https://doi.org/10.1007/s10967-013-2845-8

U. S. Environmental Protection Agency (USEPA), (1999). Radon. http://www.epa.gov/radon/ Retrieved 19/01/2017.

UNSCEAR (2008). United Nations Scientific of Committee on the Effect of atomic Radiation. Sources and Effects of Ionizing Radiation. Report to the General Assembly with Scientific Annexes. United Nations, New York.

WHO (2011). Handbook on Indoor Radon: A Public Health Perspective. WHO Guidelines Approved by the Guidelines Review Committee. Geneva

Published
2023-05-27
How to Cite
Abdulkadir M., Garba N. N., Rabiu N., Abdallah C. A. C., Saleh M. A., Abdullahi I. M., Saidu A., & Abdulkadir A. (2023). STATISTICAL ANALYSIS OF RADON CONCENTRATION IN BOREHOLE WATERS; CORRELATION TO GEOLOGICAL FORMATIONS KATSINA STATE, NORTH WESTERN NIGERIA. FUDMA JOURNAL OF SCIENCES, 7(3), 22 - 28. https://doi.org/10.33003/fjs-2023-0703-1772

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